Thought I'd chime in with an update. The volt-mod went very well; I used a pencil to increase voltage from 1.08 (stock) to 1.25. I am currently at 750Mhz on the core (stock is 625) and can run Furmark and ATI Tool artifact checker for hours with no problems. I had it at 775mhz for about an hour with no problems but it errors if it runs much more than that.
I log everything with Rivatuner and my temps have never gone above 52C even after a few hours of COD: W@W or Crysis (tried both Warhead and Vanilla). No issues with Fallout 3 either. The S1 has a 120mm fan strapped to it, so I'm sure that's helping things quite a bit. The one thing I did notice was that at this higher core speed, my memory is about 5C warmer than it was before the mod but it's still topping out at 60C, so I'm not worried about it at all.
I'm definitely CPU limited at this point and am getting ready to drop in an X4 920 in a month or so and then the hunt for 800+ is on! I see no reason why I can't get this to 1.3/1.35v on the core with the cooling that I have. I left the memory voltage at stock as I really see no reason to mess with it as much. Also, from what I've read, memory can be very easy to kill with voltage, so I figure I'll get it to what it can handle at stock and leave it at that.