yes, the way to maximize your production is one smp, 1 core for the gpu2 client, and one core to just crunch the regular way. you can't do two smp clients effectively using win xp.
You can't designate specific cores with either client. They just spread themselves out as they see fit.
I got more points per day when I ran a single SMP, but it might just depend on which WUs are crunching. I'd keep it like you have it if that is giving you the biggest PPD.
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